Adelaide Research & Scholarship
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https://hdl.handle.net/2440/74719
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| Type: | Journal article |
| Title: | Total synthesis of (+)-aureol |
| Author: | Kuan, K. Pepper, H. Bloch, W. George, J. |
| Citation: | Organic Letters, 2012; 14(18):4710-4713 |
| Publisher: | Amer Chemical Soc |
| Issue Date: | 2012 |
| ISSN: | 1523-7060 1523-7052 |
| Statement of Responsibility: | Kevin K. W. Kuan, Henry P. Pepper, Witold M. Bloch, and Jonathan H. George |
| Abstract: | A total synthesis of the marine sponge meroterpenoid (+)-aureol has been achieved in 12 steps (6% overall yield) from (+)-sclareolide. Key steps of the synthesis include a biosynthetically inspired sequence of 1,2-hydride and methyl shifts, and a biomimetic cycloetherification reaction. |
| Keywords: | Animals Porifera Diterpenes Sesquiterpenes Marine Biology Molecular Structure Stereoisomerism |
| Rights: | ©2012 American Chemical Society |
| DOI: | 10.1021/ol301715u |
| Published version: | http://dx.doi.org/10.1021/ol301715u |
| Appears in Collections: | Aurora harvest Chemistry publications IPAS publications |
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