Please use this identifier to cite or link to this item:
https://hdl.handle.net/2440/133394
Citations | ||
Scopus | Web of Science® | Altmetric |
---|---|---|
?
|
?
|
Full metadata record
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Zhang, J. | - |
dc.contributor.author | Li, Y. | - |
dc.contributor.author | Zhao, X. | - |
dc.contributor.author | Wang, L. | - |
dc.contributor.author | Chen, H. | - |
dc.contributor.author | Wang, S. | - |
dc.contributor.author | Xu, X. | - |
dc.contributor.author | Shi, L. | - |
dc.contributor.author | Zhang, L.C. | - |
dc.contributor.author | Zhu, Y. | - |
dc.contributor.author | Zhang, H. | - |
dc.contributor.author | Liu, Y. | - |
dc.contributor.author | Nealon, G. | - |
dc.contributor.author | Zhang, S. | - |
dc.contributor.author | Wu, M. | - |
dc.contributor.author | Wang, S. | - |
dc.contributor.author | Sun, H. | - |
dc.date.issued | 2021 | - |
dc.identifier.citation | Nano Energy, 2021; 89:1-11 | - |
dc.identifier.issn | 2211-2855 | - |
dc.identifier.issn | 2211-3282 | - |
dc.identifier.uri | https://hdl.handle.net/2440/133394 | - |
dc.description.abstract | Photocatalysis is essentially triggered by the photoinduced charge carriers, which are then oriented for the targeted redox reactions. However, the effects of intrinsic driving forces on charge carriers and their resulting photocatalytic throughputs remain unclear. Herein, we focus on two main potential differences (PDs), e.g., intralayer PD (IPD) within two-dimensional carbon nitride hybrids, and band PD (BPD) between the band positions of a semiconductor and the redox potentials of reactants that can actuate charge carriers for photocatalysis. In situ experiments and theoretical computations identify and differentiate the roles of the two PDs on the separation, transportation and catalytic utilization of charge carriers. It is noteworthy that the enhancement from PDs alignment in this work is higher than other physiochemical modifications (e.g., mass transfer and polymerization degree) for photocatalysis. This study may offer a guiding principle for aligning a photocatalyst with target reactions for energy conversion and chemical synthesis. | - |
dc.description.statementofresponsibility | Jinqiang Zhang, Yunguo Li, Xiaoli Zhao, Liang Wang, Haijun Chen, Shuaijun Wang ... et al. | - |
dc.language.iso | en | - |
dc.publisher | Elsevier | - |
dc.rights | © 2021 Elsevier Ltd. All rights reserved. | - |
dc.source.uri | http://dx.doi.org/10.1016/j.nanoen.2021.106357 | - |
dc.subject | Potential difference; charge carriers; carbon nitride; intralayer homojunctions; photocatalysis | - |
dc.title | Aligning potential differences within carbon nitride based photocatalysis for efficient solar energy harvesting | - |
dc.type | Journal article | - |
dc.identifier.doi | 10.1016/j.nanoen.2021.106357 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DP170104264 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DP190103548 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/LE120100026 | - |
pubs.publication-status | Published | - |
dc.identifier.orcid | Wang, S. [0000-0002-1751-9162] | - |
Appears in Collections: | Chemistry and Physics publications |
Files in This Item:
There are no files associated with this item.
Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.