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https://hdl.handle.net/2440/120740
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Type: | Journal article |
Title: | Highly efficient and stable negative electrode for asymmetric supercapacitors based on graphene/FeCo₂O₄ nanocomposite hybrid material |
Other Titles: | Highly efficient and stable negative electrode for asymmetric supercapacitors based on graphene/FeCo(2)O(4) nanocomposite hybrid material |
Author: | Chodankar, N. Dubal, D. Ji, S. Kim, D. |
Citation: | Electrochimica Acta, 2019; 295:195-203 |
Publisher: | Elsevier |
Issue Date: | 2019 |
ISSN: | 0013-4686 1873-3859 |
Statement of Responsibility: | Nilesh R. Chodankar, Deepak P. Dubal, Su-Hyeon Ji, Do-Heyoung Kim |
Abstract: | The integration of two-dimensional (2D) reduced graphene oxide (rGO) and binary metal oxide in a single electrode for asymmetric supercapacitors (ASC) is promising for overcoming the challenges driven by increasing energy-storage demands. In present work, we proposed a novel rGO/FeCo₂O₄ hybrid electrode as a negative electrode for asymmetric supercapacitors (ASC). Briefly, we engineered 3-dimensional nanocomposite materials by decorating FeCo₂O₄ nanoparticles on rGO nanosheets using facile strategy. Owing to the strong chemical bonding between the FeCo₂O₄ nanoparticles and rGO nanosheets, as-prepared rGO/FeCo₂O₄ hybrid electrode shows an ultrahigh specific capacitance of 1710 F/g on the negative potential side. Later, asymmetric supercapacitor was assembled using MnO₂ nanowires as positive electrode and rGO/FeCo₂O₄ hybrid as negative electrode, respectively. The proposed device achieved a maximum specific capacitance of 260 F/g with a specific energy of 67.5 Wh/kg and exhibited excellent cycling performance (96.02% capacity retention after 5000 cycles). Thus, the proposed design of the high-energy ASC is promising for next-generation energy-storage devices being developed for modern consumer applications. |
Keywords: | Hybrid electrode; asymmetric supercapacitor; negative electrode; ultrahigh energy density |
Rights: | © 2018 Elsevier Ltd. All rights reserved. |
DOI: | 10.1016/j.electacta.2018.10.125 |
Published version: | http://dx.doi.org/10.1016/j.electacta.2018.10.125 |
Appears in Collections: | Aurora harvest 8 Chemical Engineering publications |
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