Please use this identifier to cite or link to this item: https://hdl.handle.net/2440/117737
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dc.contributor.authorKang, J.en
dc.contributor.authorDuan, X.en
dc.contributor.authorWang, C.en
dc.contributor.authorSun, H.en
dc.contributor.authorTan, X.en
dc.contributor.authorTade, M.en
dc.contributor.authorWang, S.en
dc.date.issued2018en
dc.identifier.citationChemical Engineering Journal, 2018; 332:398-408en
dc.identifier.issn1385-8947en
dc.identifier.issn1873-3212en
dc.identifier.urihttp://hdl.handle.net/2440/117737-
dc.description.abstractNitrogen-doped bamboo-like carbon nanotubes encapsulated with nickel nanoparticles (Ni@NCNTs) were feasibly fabricated by a one-pot pyrolysis route. The characterization techniques revealed the surface morphology, structure and chemical composition of the as-prepared catalysts synthesized in different conditions. Ni@NCNTs were employed as both adsorbents and catalysts for activating persulfate to remove an emerging pollutant, antibiotic sulfachloropyridazine. The nitrogen modification enhanced both adsorption capacity and catalytic ability of Ni@NCNTs and proved to be a promising alternative to metal oxides and other carbon catalysts. Moreover, Ni@NCNTs showed an excellent stability because of nitrogen heteroatom doping and Ni nanoparticle encapsulation. Electron paramagnetic resonance (EPR) and classical radical quenching tests discovered a simultaneous radical/non-radical mechanism in Ni@NCNTs/persulfate system. The results indicated that the novel nano-architectured catalyst materials can show emerging functionalities for environmental remediation processes.en
dc.description.statementofresponsibilityJian Kang, Xiaoguang Duan, Chen Wang, Hongqi Sun, Xiaoyao Tan, Moses O. Tade, Shaobin Wangen
dc.language.isoenen
dc.publisherElsevieren
dc.rights© 2017 Elsevier B.V. All rights reserved.en
dc.subjectNitrogen doping; carbon nanotubes; antibiotics; persulfate; sulfate radicalsen
dc.titleNitrogen-doped bamboo-like carbon nanotubes with Ni encapsulation for persulfate activation to remove emerging contaminants with excellent catalytic stabilityen
dc.typeJournal articleen
dc.identifier.doi10.1016/j.cej.2017.09.102en
dc.relation.granthttp://purl.org/au-research/grants/arc/DP150103026en
pubs.publication-statusPublisheden
dc.identifier.orcidDuan, X. [0000-0001-9635-5807]en
dc.identifier.orcidWang, S. [0000-0002-1751-9162]en
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